13 research outputs found
Electrically driven convection in a thin annular film undergoing circular Couette flow
We investigate the linear stability of a thin, suspended, annular film of
conducting fluid with a voltage difference applied between its inner and outer
edges. For a sufficiently large voltage, such a film is unstable to
radially-driven electroconvection due to charges which develop on its free
surfaces. The film can also be subjected to a Couette shear by rotating its
inner edge. This combination is experimentally realized using films of smectic
A liquid crystals. In the absence of shear, the convective flow consists of a
stationary, azimuthally one-dimensional pattern of symmetric, counter-rotating
vortex pairs. When Couette flow is applied, an azimuthally traveling pattern
results. When viewed in a co-rotating frame, the traveling pattern consists of
pairs of asymmetric vortices. We calculate the neutral stability boundary for
arbitrary radius ratio and Reynolds number of the shear
flow, and obtain the critical control parameter and the critical azimuthal mode number . The
Couette flow suppresses the onset of electroconvection, so that . The calculated suppression is
compared with experiments performed at and .Comment: 17 pages, 2 column with 9 included eps figures. See also
http://mobydick.physics.utoronto.c
The adjoint problem in the presence of a deformed surface: the example of the Rosensweig instability on magnetic fluids
The Rosensweig instability is the phenomenon that above a certain threshold
of a vertical magnetic field peaks appear on the free surface of a horizontal
layer of magnetic fluid. In contrast to almost all classical hydrodynamical
systems, the nonlinearities of the Rosensweig instability are entirely
triggered by the properties of a deformed and a priori unknown surface. The
resulting problems in defining an adjoint operator for such nonlinearities are
illustrated. The implications concerning amplitude equations for pattern
forming systems with a deformed surface are discussed.Comment: 11 pages, 1 figur
Annular electroconvection with shear
We report experiments on convection driven by a radial electrical force in
suspended annular smectic A liquid crystal films. In the absence of an
externally imposed azimuthal shear, a stationary one-dimensional (1D) pattern
consisting of symmetric vortex pairs is formed via a supercritical transition
at the onset of convection. Shearing reduces the symmetries of the base state
and produces a traveling 1D pattern whose basic periodic unit is a pair of
asymmetric vortices. For a sufficiently large shear, the primary bifurcation
changes from supercritical to subcritical. We describe measurements of the
resulting hysteresis as a function of the shear at radius ratio . This simple pattern forming system has an unusual combination of
symmetries and control parameters and should be amenable to quantitative
theoretical analysis.Comment: 12 preprint pages, 3 figures in 2 parts each. For more info, see
http://mobydick.physics.utoronto.c
Weakly Nonlinear Analysis of Electroconvection in a Suspended Fluid Film
It has been experimentally observed that weakly conducting suspended films of
smectic liquid crystals undergo electroconvection when subjected to a large
enough potential difference. The resulting counter-rotating vortices form a
very simple convection pattern and exhibit a variety of interesting nonlinear
effects. The linear stability problem for this system has recently been solved.
The convection mechanism, which involves charge separation at the free surfaces
of the film, is applicable to any sufficiently two-dimensional fluid. In this
paper, we derive an amplitude equation which describes the weakly nonlinear
regime, by starting from the basic electrohydrodynamic equations. This regime
has been the subject of several recent experimental studies. The lowest order
amplitude equation we derive is of the Ginzburg-Landau form, and describes a
forward bifurcation as is observed experimentally. The coefficients of the
amplitude equation are calculated and compared with the values independently
deduced from the linear stability calculation.Comment: 26 pages, 2 included eps figures, submitted to Phys Rev E. For more
information, see http://mobydick.physics.utoronto.c
Bifurcations in annular electroconvection with an imposed shear
We report an experimental study of the primary bifurcation in
electrically-driven convection in a freely suspended film. A weakly conducting,
submicron thick smectic liquid crystal film was supported by concentric
circular electrodes. It electroconvected when a sufficiently large voltage
was applied between its inner and outer edges. The film could sustain rapid
flows and yet remain strictly two-dimensional. By rotation of the inner
electrode, a circular Couette shear could be independently imposed. The control
parameters were a dimensionless number , analogous to the Rayleigh
number, which is and the Reynolds number of the
azimuthal shear flow. The geometrical and material properties of the film were
characterized by the radius ratio , and a Prandtl-like number . Using measurements of current-voltage characteristics of a large number of
films, we examined the onset of electroconvection over a broad range of
, and . We compared this data quantitatively to
the results of linear stability theory. This could be done with essentially no
adjustable parameters. The current-voltage data above onset were then used to
infer the amplitude of electroconvection in the weakly nonlinear regime by
fitting them to a steady-state amplitude equation of the Landau form. We show
how the primary bifurcation can be tuned between supercritical and subcritical
by changing and .Comment: 17 pages, 12 figures. Submitted to Phys. Rev. E. Minor changes after
refereeing. See also http://mobydick.physics.utoronto.c
Atomistic modelling of large-scale metal film growth fronts
We present simulations of metallization morphologies under ionized sputter
deposition conditions, obtained by a new theoretical approach. By means of
molecular dynamics simulations using a carefully designed interaction
potential, we analyze the surface adsorption, reflection, and etching reactions
taking place during Al physical vapor deposition, and calculate their relative
probability. These probabilities are then employed in a feature-scale
cellular-automaton simulator, which produces calculated film morphologies in
excellent agreement with scanning-electron-microscopy data on ionized sputter
deposition.Comment: RevTeX 4 pages, 2 figure